Exogenous tetrahydrobiopterin causes endothelium-dependent contractions in isolated canine basilar artery. Kinoshita, H., and Z. S. Katusic. Departments of Anesthesiology and Pharmacology, Mayo Clinic and Mayo Foundation, 200 First Street SW, Rochester, MN 55905
APStracts 2:0561H, 1995.
Tetrahydrobiopterin is an essential cofactor in biosynthesis of nitric oxide. In contrast, in the presence of oxygen autooxidation of tetrahydrobiopterin leads to production of superoxide anions and subsequent chemical inactivation of nitric oxide. Because of these apparent opposing effects of tetrahydrobiopterin on nitric oxide levels, the present experiments were designed to determine the effect of exogenous tetrahydrobiopterin on isolated canine basilar arteries. Rings with and without endothelium were suspended for isometric force recording in modified Krebs-Ringer bicarbonate solution bubbled with 94% O2 -6% CO2 (37 degrees C, pH 7.4 ). A radioimmuno-assay technique was used to measure production of cyclic GMP. Tetrahydrobiopterin (10-7 to 10-4M), but not dihydrobiopterin or biopterin, caused endothelium-dependent contractions. Superoxide dismutase (150 U/ml) abolished tetrahydrobiopterin-induced contractions. A hydrogen peroxide scavenger catalase (1200 U/ml), and hydroxyl radical scavengers deferoxamine (10-4M) and DMSO (10-4 to 10-3M) did not significantly affect contractions to tetrahydrobiopterin. A cyclooxygenase inhibitor indomethacin (10-5M) significantly reduced the contractile effect of tetrahydrobiopterin. In the presence of a prostaglandin H2 / thromboxane A2 receptor antagonist SQ 29548 (10 -6M), contractions to tetrahydrobiopterin reversed to relaxations. In rings with endothelium, tetrahydrobiopterin (10-4M) significantly decreased the levels of cyclic GMP. These studies suggest that autooxidation of exogenous tetrahydrobiopterin induces endothelium -dependent contractions by 1) chemical inactivation of nitric oxide by superoxide anions, 2) activation of arachidonic acid metabolism via cyclooxygenase pathway with subsequent release of endoperoxide and/or thromboxane A2 from endothelial cells.

Received 1 September 1995; accepted in final form 6 December
1995.
APS Manuscript Number H828-5.
Article publication pending Am. J. Physiol. (Heart Circ. Physiology).
ISSN 1080-4757 Copyright 1995 The American Physiological Society.
Published in APStracts on 23 December 95